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Synthesis of two conjugated polymers ..
Two donor-acceptor alternating conjugated copolymers were synthesized as the donor materials of the active layer in polymer solar cells via Stille coupling reaction. Both copolymers consisted of dithienosilole as the donor unit and nonfluorinated 2,1,3-benzooxadiazole or fluorinated 2,1,3-benzooxadiazole as the acceptor unit. The nonfluorinated polymer and fluorinated polymer were designated as P1 and P2, respectively. The structures of copolymers were confirmed by FT-IR, 1H NMR, and 13C NMR. Optoelectronic properties of the polymer were investigated and observed by UV-vis spectrum, photoluminescence spectrum, and cyclic voltammetry. Both polymers exhibited a panchromatic absorption ranging from 300 nm to 1100 nm and displayed low band gaps of 1.46 eV and 1.42 eV, respectively. Both of the synthesized materials were used as the donor material in the bulk heterojunction (BHJ) solar cells and then power conversion efficiency (PCE) measurements were conducted in different weight ratios of the polymer:PC61BM blends.
The stability of the conjugated polymer-fullerene solar cell ..
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